1. 核工业北京地质研究院国家原子能机构高放废物地质处置创新中心
2. 哈尔滨工业大学环境学院
3. 南方科技大学环境科学与工程学院
网络首发:2024-08-07,
纸质出版:2025
移动端阅览
李杰彪, 周志超, 郭永海, 等. 高放废物处置北山预选区地下水化学形成机制模拟研究[J]. 地质科技通报, 2025,44(4):340-353.
李杰彪, 周志超, 郭永海, et al. 高放废物处置北山预选区地下水化学形成机制模拟研究[J]. Bulletin of Geological Science and Technology, 2025, 44(4): 340-353.
李杰彪, 周志超, 郭永海, 等. 高放废物处置北山预选区地下水化学形成机制模拟研究[J]. 地质科技通报, 2025,44(4):340-353. DOI: 10.19509/j.cnki.dzkq.tb20240194.
李杰彪, 周志超, 郭永海, et al. 高放废物处置北山预选区地下水化学形成机制模拟研究[J]. Bulletin of Geological Science and Technology, 2025, 44(4): 340-353. DOI: 10.19509/j.cnki.dzkq.tb20240194.
研究地下水化学特性对于高放废物处置库选址和长期性能安全评价是十分必要的。采用水文地球化学综合分析和模拟方法,探讨了我国高放废物处置库预选区甘肃北山地区基岩裂隙水的基本化学特征、水平分带性以及不同水文地质区水化学形成机制。结果表明:区内地下水化学类型主要为Cl·SO
4
-Na型和SO
4
·Cl-Na型,pH值多在7.5~8.3之间。基岩裂隙水对岩盐、石膏、萤石、绿泥石以及长石类等矿物多处于未饱和状态,而对黏土类矿物则多处于过饱和状态。从补给区到排泄区,基岩裂隙水化学分布表现出较为明显的水平分带性。马鬃山一带是区域地下水主要补给区,地下水矿化度低,水化学组分形成主要受溶滤作用控制;沉积盆地是地下水主要排泄区,地下水矿化度高,水化学组分形成主要受蒸发作用控制;在径流区,地下水化学形成主要受岩盐、石膏等矿物的溶解控制,而碳酸盐类和硅酸盐类矿物的溶解或沉淀作用微弱。该区基岩裂隙水化学形成主要受蒸发浓缩作用及水-岩相互作用的影响和控制,该结果为高放废物处置库选址提供了地下水化学基础信息和数据。
ObjectiveHydrogeochemical characteristics play a pivotal role in site selection and long-term safety assessment for high-level radioactive waste (HLW) disposal repositories. MethodsThis study employs integrated hydrogeochemical analysis and modeling to investigate the basic hydrogeochemical characteristics
horizontal zoning
and formation mechanisms in different hydrogeological zones of the Beishan preselected site for HLW disposal in Gansu Province
China. ResultsThe results show that the predominant hydrogeochemical types were Cl·SO4-Na and SO4·Cl-Na
Province with pH values generally ranging from 7.5 to 8.3. Fractured bedrock groundwater is typically undersaturated with respect to halite
gypsum
fluorite
glauconite
and feldspar
and oversaturated with respect to clay minerals. A distinct horizontal zonation is observed in the hydrogeochemical composition from the recharge area to the discharge area. The Mazongshan region serves as the primary recharge zone
characterized by low mineralization
where hydrogeochemical composition is mainly controlled by leaching processes. The sedimentary basins act as the main discharge areas with high mineralization
where evaporation processes dominate. The water-rock interaction processes along the flow path are primarily driven by the dissolution of halite and gypsum
while the effect of carbonate and silicate dissolution or precipitation remains relatively weak. ConclusionOverall
the hydrogeochemical formation of fractured bedrock groundwater in the Beishan area is predominantly governed by evaporation and water-rock interaction processes. This study provides fundamental hydrogeochemical data and insights to support the site selection of the HLW disposal repository.
范芷若.再生水灌溉条件下的地下水水质分析及水文地球化学模拟[D].长安大学,2024(07).
李仁海.甘肃北山钻孔地下水流速流向测定及地下水流数值模拟[D].成都理工大学,2020(04).
马文静,王文科,侯昕悦,季德帅,马稚桐.玛纳斯河流域河水-地下水转化驱动下的水文地球化学空间演化[J].地质科技通报,2025(02).
李杰彪,梁修雨,周志超,赵敬波,潘跃龙,郭永海.某地下核设施场址地下水化学特征及其对水循环的指示意义[J].地球科学,2024(03).
袁昊辰,张幼宽,梁修雨.广州某地下水污染场地监控自然衰减修复模拟[J].地质科技通报,2023(04).
李杰彪,周志超,云龙,苏锐,郭永海.基于土壤氡气测量识别甘肃北山南缘隐伏断裂[J].地质学报,2022(06).
王驹.中国高放废物地质处置21世纪进展[J].原子能科学技术,2019(10).
Ju Wang,Liang Chen,Rui Su,Xingguang Zhao.The Beishan underground research laboratory for geological disposal of high-level radioactive waste in China:Planning, site selection,site characterization and in situ tests[J].Journal of Rock Mechanics and Geotechnical Engineering,2018(03).
郭永海,王海龙,董建楠,苏锐,刘淑芬,周志超.高放废物处置库芨芨槽预选场址深部地下水同位素研究[J].地质学报,2013(09).
郭永海,王驹,肖丰,王志明,刘淑芬,苏锐,宗自华,李亚伟,王海龙.高放废物处置库甘肃北山预选区地下水的形成[J].高校地质学报,2010(01).
郭永海,王驹,萧丰,王志明,刘淑芬,苏锐,宗自华.高放废物处置库北山预选区地下水同位素组成特征及其意义[J].地球学报,2008(06).
郭永海,王驹.高放废物地质处置中的地质、水文地质、地球化学关键科学问题[J].岩石力学与工程学报,2007(S2).
王驹,陈伟明,苏锐,郭永海,金远新.高放废物地质处置及其若干关键科学问题[J].岩石力学与工程学报,2006(04).
郭永海,王驹,吕川河,刘淑芬,钟自华.高放废物处置库甘肃北山野马泉预选区地下水化学特征及水-岩作用模拟[J].地学前缘,2005(S1).
王丽,王金生,林学钰.水文地球化学模型研究进展[J].水文地质工程地质,2003(06).
郭永海,沈照理,钟佐燊.河北平原地下水化学环境演化的地球化学模拟[J].中国科学(D辑:地球科学),1997(04).
Li Jiebiao,Zhang You-Kuan,Zhou Zhichao,Guo Yonghai,Zhao Jingbo,Liang Xiuyu.Using multiple isotopes to determine groundwater source, age, and renewal rate in the Beishan preselected area for geological disposal of high-level radioactive waste in China[J].Journal of Hydrology,2024.
Fu Yunmei,Dong Yanhui,Wang Liheng,Bour Olivier,Klepikova Maria V.,Zong Zihua,Xu Zhifang,Zhou Zhichao.Characteristics of hydraulic conductivity in mountain block systems and its effects on mountain block recharge: Insights from field investigation and numerical modeling[J].Journal of Hydrology,2022.
Li Lulu,Zhang Qiulan,Zhou Zhichao,Cui Yali,Shao Jingli,Zhao Yu.Groundwater circulation patterns in bedrock aquifers from a pre-selected area of high-level radioactive waste repository based on two-dimensional numerical simulation[J].Journal of Hydrology,2022.
Ju Qiding,Hu Youbiao,Liu Qimeng,Liu Yu,Hu Taifeng.Key hydrological process of a multiple aquifer flow system in the mining area of Huaibei plain, Eastern China[J].Applied Geochemistry,2022.
Christos Christofi,Adriana Bruggeman,Christoph Kuells,Costas Constantinou.Hydrochemical evolution of groundwater in gabbro of the Troodos Fractured Aquifer. A comprehensive approach[J].Applied Geochemistry,2020.
Haitao Zhang,Guangquan Xu,Hongbin Zhan,Xiaoqing Chen,Mancai Liu,Minhua Wang.Identification of hydrogeochemical processes and transport paths of a multi-aquifer system in closed mining regions[J].Journal of Hydrology,2020.
Andres Marandi,Paul Shand.Groundwater chemistry and the Gibbs Diagram[J].Applied Geochemistry,2018.
Pu Liu,Nils Hoth,Carsten Drebenstedt,Yajun Sun,Zhimin Xu.Hydro-geochemical paths of multi-layer groundwater system in coal mining regions — Using multivariate statistics and geochemical modeling approaches[J].Science of the Total Environment,2017.
Cüneyt Güler,Geoffrey D. Thyne,Hidayet Ta?a,ümit Y?ld?r?m.Processes Governing Alkaline Groundwater Chemistry within a Fractured Rock (Ophiolitic Mélange) Aquifer Underlying a Seasonally Inhabited Headwater Area in the Alada?lar Range (Adana, Turkey)[J].Geofluids,2017.
J. Morán-Ramírez,R. Ledesma-Ruiz,J. Mahlknecht,J.A. Ramos-Leal.Rock–water interactions and pollution processes in the volcanic aquifer system of Guadalajara, Mexico, using inverse geochemical modeling[J].Applied Geochemistry,2016.
Didier Gastmans,Ian Hutcheon,Amauri Antônio Menegário,Hung Kiang Chang.Geochemical evolution of groundwater in a basaltic aquifer based on chemical and stable isotopic data: Case study from the Northeastern portion of Serra Geral Aquifer, São Paulo state (Brazil)[J].Journal of Hydrology,2016.
Chin‐Fu Tsang,Ivars Neretnieks,Yvonne Tsang.Hydrologic issues associated with nuclear waste repositories[J].Water Resources Research,2015.
Bianchi Marco,Liu Hui-Hai,Birkholzer Jens T.Radionuclide transport behavior in a generic geological radioactive waste repository.[J].Ground water,2015.
María J. Gimeno,Luis F. Auqué,Patricia Acero,Javier B. Gómez.Hydrogeochemical characterisation and modelling of groundwaters in a potential geological repository for spent nuclear fuel in crystalline rocks (Laxemar, Sweden)[J].Applied Geochemistry,2014.
Kyu-Youl Sung,Seong-Taek Yun,Maeng-Eon Park,Yong-Kwon Koh,Byoung-Young Choi,Ian Hutcheon,Kyoung-Ho Kim.Reaction path modeling of hydrogeochemical evolution of groundwater in granitic bedrocks, South Korea[J].Journal of Geochemical Exploration,2012.
Marcus Laaksoharju,John Smellie,Eva-Lena Tullborg,María Gimeno,Jorge Molinero,Ioana Gurban,Lotta Hallbeck.Hydrogeochemical evaluation and modelling performed within the Swedish site investigation programme[J].Applied Geochemistry,2008.
Marcus Laaksoharju,Mel Gascoyne,Ioana Gurban.Understanding groundwater chemistry using mixing models[J].Applied Geochemistry,2008.
Lipson David S,McCray John E,Thyne Geoffrey D.Using PHREEQC to simulate solute transport in fractured bedrock.[J].Ground water,2007.
M.U. Sharif,R.K. Davis,K.F. Steele,B. Kim,T.M. Kresse,J.A. Fazio.Inverse geochemical modeling of groundwater evolution with emphasis on arsenic in the Mississippi River Valley alluvial aquifer, Arkansas (USA)[J].Journal of Hydrology,2007.
Gi-Tak Chae,Seong-Taek Yun,Kangjoo Kim,Bernhard Mayer.Hydrogeochemistry of sodium-bicarbonate type bedrock groundwater in the Pocheon spa area, South Korea: water–rock interaction and hydrologic mixing[J].Journal of Hydrology,2005.
Pierre D. Glynn,L. Niel Plummer.Geochemistry and the understanding of ground-water systems[J].Hydrogeology journal,2005.
Cüneyt Güler,Geoffrey D. Thyne,John E. McCray,Keith A. Turner.Evaluation of graphical and multivariate statistical methods for classification of water chemistry data[J].Hydrogeology Journal,2002.
Jozsef Toth.Groundwater as a geololgic agent: An overview of the causes, processes, and manifestations[J].Hydrogeology journal,1999.
Gibbs R J.Mechanisms Controlling World Water Chemistry[J].Science (New York, N.Y.),1970.
0
浏览量
235
下载量
3
CSCD
关联资源
相关文章
相关作者
相关机构
京公网安备11010802024621