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宋镇泽, 牛大伟, 薛爽, et al. Analysis of Pollution Characteristics and Sources of VOCs in Autumn in Urban Area of Luohe City[J]. 2024, 47(S1): 86-94.
宋镇泽, 牛大伟, 薛爽, et al. Analysis of Pollution Characteristics and Sources of VOCs in Autumn in Urban Area of Luohe City[J]. 2024, 47(S1): 86-94. DOI: 10.19672/j.cnki.1003-6504.0840.23.338.
该文利用2021年11月5-11日漯河市3个市区点位环境挥发性有机物(VOCs)手工采样数据,开展VOCs污染特征和来源解析,识别臭氧生成潜势(OFP)和二次有机气溶胶生成潜势(SOAFP)的关键物种及污染源。结果表明,监测期间漯河市TVOC平均体积分数为51×10~(-9),以OVOCs(36.1%)和烷烃(30.7%)贡献为主,空间变化为三五一五工厂水利局卫健委。OFP均值为348.8μg/m~3,各点位贡献前10物种以芳香烃和OVOCs为主,移动源是贡献最高的排放源;SOAFP均值为1.8μg/m~3,各点位均为芳香烃贡献最大,移动源是主要贡献源类。正定矩阵因子模型解析结果显示,移动源(25.4%)、油气挥发源(18.9%)、溶剂使用源(18.6%)、工业排放源(17.5%)和燃烧源(15.1%)是市区大气VOCs主要排放源。
张远航.中国大气臭氧污染防治蓝皮书(2020年)[M].2020.Zhang Yuanhang. Blue Book on Prevention and Control of Atmospheric Ozone Pollution in China(in Chinese)[M]. Beijing:Science Press, 2020.
姜华,高健,李红,等.我国大气污染协同防控理论框架初探[J].环境科学研究, 2022,35(3):601-610.Jiang Hua, Gao Jian, Li Hong, et al. A preliminary study on the theoretical framework of coordinated prevention and control of air pollution in China[J]. Research of Environmental Sciences, 2022,35(3):601-610.
李嫣,王浙明,宋爽,等.化学合成类制药行业工艺废气VOCs排放特征与危害评估分析[J].环境科学, 2014,35(10):3663-3668.Li Yan, Wang Zheming, Song Shuang, et al. Characteristics and hazard assessment of VOCs emission from process waste gas in chemical synthesis pharmaceutical industry[J].Environmental Science, 2014,35(10):3663-3668.
Huang X F, Dai J, Zhu Q, et al. Abundant biogenic oxygenated organic aerosol in atmospheric coarse particles:plausible sources and atmospheric implications[J]. Environmental Science and Technology, 2020,54(3):1425-1430.
Liu Y F, Song M D, Liu X G, et al. Characterization and sources of volatile organic compounds(VOCs)and their related changes during ozone pollution days in 2016 in Beijing,China[J]. Environmental Pollution, 2020,257:113599.
Wei W, Li Y, Wang Y T, et al. Characteristics of VOCs during haze and non-haze days in Beijing, China:concentration, chemical degradation and regional transport impact[J].Atmospheric Environment, 2018,194:134-145.
Liu B S, Liang D N, Yang J M, et al. Characterization and source apportionment of volatile organic compounds based on 1-year of observational data in Tianjin, China[J]. Environmental Pollution, 2016,218:757-769.
Gao Y Q, Li M, Wan X, et al. Important contributions of alkenes and aromatics to VOCs emissions, chemistry and secondary pollutants formation at an industrial site of central Eastern China[J]. Atmospheric Environment, 2021, 244:117927.
Zheng S S, Xu X F, Zhang Y J, et al. Characteristics and sources of VOCs in urban and suburban environments in Shanghai, China, during the 2016 G20 Summit[J]. Atmospheric Pollution Research, 2019,10(6):1766-1779.
Chen C, Wang L R, Qin Y H, et al. VOC characteristics and their source apportionment in the Yangtze River Delta Region during the G20 Summit[J]. Atmosphere, 2021, 12(7):928.
Jia H H, Gao S, Duan Y S, et al. Investigation of health risk assessment and odor pollution of volatile organic compounds from industrial activities in the Yangtze River Delta Region, China[J]. Ecotoxicology and Environmental Safety,2021,208:111474.
He Z R, Wang X M, Ling Z H, et al. Contributions of different anthropogenic volatile organic compound sources to ozone formation at a receptor site in the Pearl River Delta Region and its policy implications[J]. Atmospheric Chemistry and Physics, 2019,19(13):8801-8816.
Meng Y, Song J W, Zeng L W, et al. Ambient volatile organic compounds at a receptor site in the Pearl River Delta Region:variations, source apportionment and effects on ozone formation[J]. Journal of Environmental Sciences, 2022,111:104-117.
Tan Q W, Liu H F, Xie S D, et al. Temporal and spatial distribution characteristics and source origins of volatile organic compounds in a megacity of Sichuan Basin, China[J]. Environmental Research, 2020,185:109478.
Li L Y, Chen Y, Zeng L M, et al. Biomass burning contribution to ambient volatile organic compounds(VOCs)in the Chengdu-Chongqing Region(CCR), China[J]. Atmospheric Environment, 2014,99:403-410.
秦涛,徐勃,王信梧,等.淄博市夏季城区与背景点VOCs污染特征比较[J].环境科学, 2022,43(3):1286-1295.Qin Tao, Xu Bo, Wang Xinwu, et al. Comparison of VOCs pollution characteristics between urban areas and background points in Zibo City in summer[J]. Environmental Science, 2022,43(3):1286-1295.
贾智海,顾瑶,孔翠丽,等.青岛市臭氧污染与非污染期间VOCs化学特征及来源解析[J].环境科学, 2023,44(4):1962-1973.Jia Zhihai, Gu Yao, Kong Cuili, et al. Chemical characteristics and source analysis of VOCs during ozone pollution and non-pollution in Qingdao[J]. Environmental Science, 2023,44(4):1962-1973.
孙雪松,张蕊,王裕,等.北京市城区秋季O3污染过程VOCs污染特征及反应活性[J].环境科学, 2023,44(2):691-698.Sun Xuesong, Zhang Rui, Wang Yu, et al. Characteristics and reactivity of VOCs during O3pollution in autumn in Beijing[J]. Environmental Science, 2023,44(2):691-698.
张敬巧,吴亚君,李慧,等.廊坊开发区秋季VOCs污染特征及来源解析[J].中国环境科学, 2019,39(8):3186-3192.Zhang Jingqiao, Wu Yajun, Li Hui, et al. Characteristics and source analysis of VOCs pollution in Langfang development zone in autumn[J]. China Environmental Science, 2019, 39(8):3186-3192.
王泰,朱彬,施双双,等.南京北郊工业乡村混合区秋季边界层VOCs垂直分布特征[J].环境科学, 2023,44(1):66-74.Wang Tai, Zhu Bin, Shi Shuangshuang, et al. Vertical distribution characteristics of VOCs in autumn boundary layer in industrial and rural mixed area of northern suburb of Nanjing[J]. Environmental Science, 2023,44(1):66-74.
林旭,陈超,叶辉,等.杭州秋季大气VOCs变化特征及化学反应活性研究[J].中国环境监测, 2020,36(2):196-204.Lin Xu, Chen Chao, Ye Hui, et al. Variation characteristics and chemical reactivity of VOCs in different functional zones of Hangzhou in autumn[J]. Environmental Monitoring in China, 2020,36(2):196-204.
陈雪,黄晓锋,朱波,等.深圳市秋季VOCs空间分布特征与关键减排物种[J].中国环境科学, 2021,41(9):4069-4076.Chen Xue, Huang Xiaofeng, Zhu Bo, et al. Spatial distribution characteristics of VOCs and key emission reduction species in autumn Shenzhen[J]. China Environmental Science,2021,41(9):4069-4076.
张翼翔,尹沙沙,袁明浩,等.郑州市春季大气挥发性有机物污染特征及源解析[J].环境科学, 2019,40(10):4372-4381.Zhang Yixiang, Yin Shasha, Yuan Minghao, et al. Characteristics and source apportionment of ambient VOCs in spring in Zhengzhou[J]. Environmental Science, 2019,40(10):4372-4381.
王冰,尹沙沙,黄爱枝,等.郑州市多站点大气VOCs变化特征及源解析[J].环境科学, 2023,44(2):699-708.Wang Bing, Yin Shasha, Huang Aizhi, et al. Variation characteristics and source analysis of atmospheric VOCs at multiple stations in Zhengzhou City[J]. Environmental Science,2023,44(2):699-708.
王鸣,项萍,牛其恺,等.南阳市冬春交替期大气VOCs污染特征及来源解析[J].环境科学学报, 2018,38(6):2233-2241.Wang Ming, Xiang Ping, Niu Qikai, et al. Characteristics and source analysis of VOCs pollution in Nanyang city during the alternating period of winter and spring[J]. Acta Scientiae Circumstantiae, 2018,38(6):2233-2241.
施雨其,郑凯允,丁玮婷,等.开封市城区冬季大气挥发性有机物污染特征及来源解析[J].环境科学, 2023,44(4):1933-1942.Shi Yuqi, Zheng Kaiyun, Ding Weiting, et al. Characteristics and source analysis of volatile organic compounds pollution in winter in Kaifeng City[J]. Environmental Science,2023,44(4):1933-1942.
王剑平,靳朝喜,李辉,等.洛阳市吉利区环境空气中挥发性有机物时空分布特征研究[J].分析仪器, 2016(3):64-70.Wang Jianping, Jin Chaoxi, Li Hui, et al. Temporal and spatial distribution characteristics of volatile organic compounds in ambient air in Jili district of Luoyang City[J].Analytical Instrumentation, 2016(3):64-70.
齐一谨,倪经纬,王玲玲,等.郑州市秋季VOCs污染特征及来源解析研究[J].环境科学与技术, 2022,45(4):116-125.Qi Yijin, Ni Jingwei, Wang Lingling, et al. Characteristics and source apportionment of ambient volatile organic compounds in Zhengzhou in autumn[J]. Environmental Science&Technology, 2022,45(4):116-125.
秦涛.淄博市城区大气VOCs污染特征、环境影响及健康风险评价[D].天津:天津理工大学, 2022.Qin Tao. Pollution Characteristics, Environmental Effect and Health Risk Assessment of Ambient VOCs in Zibo City[D]. Tianjin:Tianjin University of Technology, 2022.
宋晗睿,徐勃,王健,等.我国典型工业城市夏冬季卤代烃来源解析与致癌风险[J].环境科学研究, 2022,35(11):2527-2537.Song Hanrui, Xu Bo, Wang Jian, et al. Halogenated hydrocarbon source apportionment and carcinogenic risks in summer and winter in a typical industrial city of China[J]. Research of Environmental Sciences, 2022,35(11):2527-2537.
Carter W P L. Reactivity Estimates for Selected Consumer Product Compounds[R]. 2008.
Carter W P L. Development of ozone reactivity scales for volatile organic compounds[J]. Air&Waste, 1994, 44(7):881-899.
Grosjean D, Seinfeld J H. Parameterization of the formation potential of secondary organic aerosols[J]. Atmospheric Environment(1967), 1989,23(8):1733-1747.
Grosjean D. In situ organic aerosol formation during a smog episode:estimated production and chemical functionality[J].Atmospheric Environment Part A General Topics, 1992,26(6):953-963.
Martín-Reviejo M, Wirtz K. Is benzene a precursor for secondary organic aerosol?[J]. Environmental Science and Technology, 2005,39(4):1045-1054.
Kroll J H, Ng N L, Murphy S M, et al. Secondary organic aerosol formation from isoprene photooxidation under highNOxconditions[J]. Geophysical Research Letters, 2005, 32(18):L18808, doi:10.1029/2005GL023637.
Paatero P, Tapper U. Analysis of different modes of factor analysis as least squares fit problems[J]. Chemometrics and Intelligent Laboratory Systems, 1993,18(2):183-194.
周振,肖林海,费蕾蕾,等.东莞工业集中区夏季臭氧污染与非污染期间VOCs组分特征及其来源[J].环境科学, 2022,43(9):4497-4505.Zhou Zhen, Xiao Linhai, Fei Leilei, et al. Characteristics and source apportionment of volatile organic compounds(VOCs)in a typical industrial area in Dongguan during periods of ozone and non-ozone pollution in summer[J]. Environmental Science, 2022,43(9):4497-4505.
Vestenius M, Hopke P K, Lehtipalo K, et al. Assessing volatile organic compound sources in a boreal forest using positive matrix factorization(PMF)[J]. Atmospheric Environment, 2021,259:118503.
Atkinson R, Arey J. Atmospheric degradation of volatile organic compounds[J]. ChemInform, 2004,35(10):doi:10.1002/chin. 200410285.
易宵霄,李姜豪,李光华,等.铜川市秋冬季大气VOCs特征及其O3和SOA形成潜势分析[J].环境科学, 2022,43(1):140-149.Yi Xiaoxiao, Li Jianghao, Li Guanghua, et al. Characteristics of atmospheric VOCs in Tongchuan in autumn and winter, and potential analysis of O3and SOA formation[J]. Environmental Science, 2022,43(1):140-149.
Hui L R, Liu X G, Tan Q W, et al. VOC characteristics,sources and contributions to SOA formation during haze events in Wuhan, Central China[J]. Science of the Total Environment, 2019,650:2624-2639.
林燕芬,段玉森,高宗江,等.基于VOCs加密监测的上海典型臭氧污染过程特征及成因分析[J].环境科学学报, 2019,39(1):126-133.Lin Yanfen, Duan Yusen, Gao Zongjiang, et al. Typical ozone pollution process and source identification in Shanghai based on VOCs intense measurement[J]. Acta Scientiae Circumstantiae, 2019,39(1):126-133.
景盛翱,叶旭红,高雅琴,等.典型光化学污染期间杭州大气挥发性有机物污染特征及反应活性[J].环境科学, 2020,41(7):3076-3084.Jing Sheng’ao, Ye Xuhong, Gao Yaqin, et al. Characteristics and reactivity of VOCs in Hangzhou during a typical photochemical pollution episode[J]. Environmental Science,2020,41(7):3076-3084.
Li J, Xie S D, Zeng L M, et al. Characterization of ambient volatile organic compounds and their sources in Beijing, before, during, and after Asia-Pacific Economic Cooperation China 2014[J]. Atmospheric Chemistry and Physics, 2015,15(14):7945-7959.
Li B W, Ho S S H, Gong S L, et al. Characterization of VOCs and their related atmospheric processes in a central Chinese city during severe ozone pollution periods[J]. Atmospheric Chemistry and Physics, 2019,19(1):617-638.
Liu Y, Shao M, Fu L L, et al. Source profiles of volatile organic compounds(VOCs)measured in China:part I[J]. Atmospheric Environment, 2008,42(25):6247-6260.
Song M D, Li X, Yang S D, et al. Spatiotemporal variation,sources, and secondary transformation potential of volatile organic compounds in Xi’an, China[J]. Atmospheric Chemistry and Physics, 2021,21(6):4939-4958.
Yuan B, Shao M, Lu S H, et al. Source profiles of volatile organic compounds associated with solvent use in Beijing,China[J]. Atmospheric Environment, 2010, 44(15):1919-1926.
朱玉凡,陈强,刘晓,等.基于气团老化程度对挥发性有机物分类改善PMF源解析效果[J].环境科学, 2022,43(2):707-713.Zhu Yufan, Chen Qiang, Liu Xiao, et al. Improved performance of PMF source apportionment for volatile organic compounds based on classification of VOCs’aging degree in air mass[J]. Environmental Science, 2022,43(2):707-713.
刘佳,翟崇治,余家燕,等.重庆市环境空气中VOCs的空间分布及来源解析[J].环境科学与技术, 2018,41(2):71-76.Liu Jia, Zhai Chongzhi, Yu Jiayan, et al. Source apportionment of VOCs at city center of Chongqing in summer[J]. Environmental Science&Technology, 2018,41(2):71-76.
周子航,邓也,吴柯颖,等.成都市典型工艺过程源挥发性有机物源成分谱[J].环境科学, 2019,40(9):3949-3961.Zhou Zihang, Deng Ye, Wu Keying, et al. Source profiles of VOCs associated with typical industrial processes in Chengdu[J]. Environmental Science, 2019,40(9):3949-3961.
吕大器,陆思华,邵敏,等.典型胶合板制造企业VOCs排放特征[J].中国环境科学, 2020,40(5):1924-1931.Lyu Daqi, Lu Sihua, Shao Min, et al. Emission characteristics of volatile organic compounds(VOCs)from typical plywood industry[J]. China Environmental Science, 2020,40(5):1924-1931.
Hsieh L T, Yang H H, Chen H W. Ambient BTEX and MTBE in the neighborhoods of different industrial parks in Southern Taiwan[J]. Journal of Hazardous Materials, 2006,128(2/3):106-115.
虞小芳,程鹏,古颖纲,等.广州市夏季VOCs对臭氧及SOA生成潜势的研究[J].中国环境科学, 2018,38(3):830-837.Yu Xiaofang, Cheng Peng, Gu Yinggang, et al. Formation potential of ozone and secondary organic aerosol from VOCs oxidation in summer in Guangzhou, China[J]. China Environmental Science, 2018,38(3):830-837.
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